diff --git a/.chloggen/remove-profiles-dictionary.yaml b/.chloggen/remove-profiles-dictionary.yaml
new file mode 100644
index 0000000000..b266fae791
--- /dev/null
+++ b/.chloggen/remove-profiles-dictionary.yaml
@@ -0,0 +1,25 @@
+# Use this changelog template to create an entry for release notes.
+
+# One of 'breaking', 'deprecation', 'new_component', 'enhancement', 'bug_fix'
+change_type: breaking
+
+# The name of the component, or a single word describing the area of concern, (e.g. otlpreceiver)
+component: pdata/pprofile
+
+# A brief description of the change.  Surround your text with quotes ("") if it needs to start with a backtick (`).
+note: Remove deprecated ProfilesDictionary method
+
+# One or more tracking issues or pull requests related to the change
+issues: [13858]
+
+# (Optional) One or more lines of additional information to render under the primary note.
+# These lines will be padded with 2 spaces and then inserted directly into the document.
+# Use pipe (|) for multiline entries.
+subtext:
+
+# Optional: The change log or logs in which this entry should be included.
+# e.g. '[user]' or '[user, api]'
+# Include 'user' if the change is relevant to end users.
+# Include 'api' if there is a change to a library API.
+# Default: '[user]'
+change_logs: [api]
diff --git a/pdata/pprofile/profiles.go b/pdata/pprofile/profiles.go
index 8baa522497..bda6738d46 100644
--- a/pdata/pprofile/profiles.go
+++ b/pdata/pprofile/profiles.go
@@ -3,11 +3,6 @@
 
 package pprofile // import "go.opentelemetry.io/collector/pdata/pprofile"
 
-// Deprecated: [v0.133.0] use Dictionary().
-func (ms Profiles) ProfilesDictionary() ProfilesDictionary {
-	return ms.Dictionary()
-}
-
 // MarkReadOnly marks the ResourceProfiles as shared so that no further modifications can be done on it.
 func (ms Profiles) MarkReadOnly() {
 	ms.getState().MarkReadOnly()